Johannes Karges and his team have developed a new mechanism of activity against cancer cells.
© RUB, Marquard

Medicine

Treating Tumors Independently of Oxygen

Most tumors grow so rapidly that vascular growth cannot keep up, and oxygen-depleted areas form within them. A new active agent could make it possible to treat them with photodynamic therapy.

Photodynamic treatment of cancer is based on administering an initially inactive substance that is only activated in the tumor via targeted light irradiation. It then generates reactive oxygen species that kill the cancer cells. However, this method reaches its limits when no oxygen is present, as is the case with many fast-growing tumors. Professor Johannes Karges’ research group at Ruhr University Bochum has achieved a breakthrough that makes the treatment of such tumors possible: When oxygen is absent, an alternative action mechanism comes into effect. This uses hydrogen peroxide, a natural metabolic product of the cells. The researchers report their findings in the Journal of the American Chemical Society from April 6, 2026.

An entirely new action mechanism

Photodynamic therapy, or PDT, is an established method for treating cancer and is widely used in clinical practice. Karges and his team have developed an entirely new action mechanism that functions independently of the oxygen concentration within the tissue: Light converts the ruthenium-based active agent into an excited electronic state. When oxygen is present, energy is transferred to molecular oxygen, creating singlet oxygen, which has a harmful effect on cells. “This process corresponds to the conventional, oxygen-dependent mechanism of photodynamic therapy,” says Karges.

When oxygen is absent, another mechanism comes into effect. The cause is the coordination of intracellular iron to the active agent. This interaction alters the electronic characteristics of the system such that instead of a transfer of energy, an ultra-fast, metal-to-metal transfer of electrons occurs from the excited ruthenium center to the iron center. The hydrogen peroxide is thereby converted into highly reactive hydroxyl radicals. “Because hydrogen peroxide is a natural metabolic product of the cell, this process can occur independently of the molecular oxygen,” explains Karges. The hydroxyl radicals that have formed cause oxidative damage to central cellular structures and thus kill the cancer cells.

This means that the substance remains active even under severe conditions where past therapies have failed. In the current study, the researchers demonstrated this with breast cancer cells. “This method can be used for many different types of tumors, in principle,” says Karges. “However, we have not yet begun trying this out with human subjects and are working to develop this.”

Funding

The work was funded by the Liebig Grant from the Chemical Industry Fund of Verband der Chemischen Industrie, the Life Sciences Bridge Award of the Aventis Foundation, and the Paul Ehrlich & Ludwig Darmstaedter Early Career Award 2024 (issued by the Paul Ehrlich Foundation).

Original publication

Nicolás Montesdeoca, Zisis Papadopoulos, Hung Manh Tran, Steffi Krause Hinojosa, Henrik Sielhorst, Jacqueline Heinen-Weiler, Johannes Karges: Exploiting Metal-to-Metal Electron Transfer in a Ru(II) Polypyridine–Deferasirox Conjugate for Hypoxic Photodynamic Therapy, in: Journal of the American Chemical Society, 2026, DOI: 10.1021/jacs.5c20295.

Press contact

Professor Johannes Karges
Medical Inorganic Chemistry
Faculty of Chemistry and Biochemistry, Faculty of Medicine
Ruhr University Bochum
Phone: +49 234 32 24187
Email: johannes.karges@ruhr-uni-bochum.de

Research group website
 

Download high-resolution images
The selected images are downloaded as a ZIP file. The captions and image credits are available in the HTML file after unzipping.
Conditions of use
The images are free to use for members of the press, provided the relevant copyright notice is included. The images may be used solely for press coverage of Ruhr-Universität Bochum that relates solely to the contents of the article that includes the link for the image download. By downloading the images, you receive a simple right of use for one-time reporting. Saving the images for other purposes or further processing of the images that goes beyond adapting them to the respective layout requires an extended right of use. Should you therefore wish to use the photos in any other way, please contact redaktion@ruhr-uni-bochum.de

Published

Tuesday
07 April 2026
9:53 am

By

Meike Drießen (md)

Translated by

Allround Fremdsprachen GmbH von der Lühe

Share